A thermodynamic theory on the nonlinear viscoelasticity of glassy polymers, 1: Constitutive equation

Kwang Soo Cho, Sang Yong Kim

Research output: Contribution to journalArticlepeer-review

4 Scopus citations

Abstract

We have developed a nonlinear viscoelastic constitutive equation, which can predict the yield behavior of polymers. This constitutive equation results from the viewpoints that the plastic flow of glassy polymers can be described by a soliton, which is expected to unify the existing concepts for viscoelasticity and yield of glassy polymers, such as dislocation, disclination and free volume. Although our approach is based on molecular concepts and irreversible thermodynamics, it is phenomenological.

Original languageEnglish
Pages (from-to)328-335
Number of pages8
JournalMacromolecular Theory and Simulations
Volume9
Issue number6
DOIs
StatePublished - 2000

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