Desulfurization kinetics of molten copper matte by gas bubbling

Ho Sang Sohn, Yasuhiro Fukunaka, Toshio Oishi

Research output: Chapter in Book/Report/Conference proceedingConference contributionpeer-review

3 Scopus citations

Abstract

The kinetic study on desulfurization of copper matte by gas bubbling was designed under the presumptions of lower FeO activity and of no slag formation. Copper matte with 59% Cu and 22.6% S in weight was oxidized at 1523K by bubbling of Ar + O2 gas through a submerged nozzle. The effects of oxygen partial pressure and flow rate of gas on the oxidation rate of matte were discussed. The desulfurization rate and the evolution rate of SO2 gas of copper matte were significantly influenced by the oxygen partial pressure, but the dependence on gas flow rate was rather complicated. The desulfurization rate and evolution rate of SO2 gas of copper matte were described by the mass transfer rate through the gas film around the rising gas bubbles. Thermodynamic correlation equations between the partial pressure of gaseous species and matte composition were incorporated to the kinetic calculation. The present model shows that the reaction path starts to transiently cross over an isobar line of pSO2 to asymptotically approach to the particular isobar line drawn in a matte composition plane of %S and %O.

Original languageEnglish
Title of host publicationYazawa International Symposium
Subtitle of host publicationMetallurgical and Materials Processing: Principles and Techologies; Materials Processing Fundamentals and New Technologies
EditorsF. Kongoli, K. Itagaki, C. Yamauchi, H.Y. Sohn, F. Kongoli, K. Itagaki, C. Yamauchi, H.Y. Sohn
Pages131-146
Number of pages16
StatePublished - 2003
EventYazawa International Symposium: Metallurgical and Materials Processing: Principles and Technologies; Materials Processing Fundamentals and New Technologies - San Diego, CA, United States
Duration: 2 Mar 20036 Mar 2003

Publication series

NameYazawa International Symposium: Metallurgical and Materials Processing: Principles and Techologies; Materials Processing Fundamentals and New Technologies
Volume1

Conference

ConferenceYazawa International Symposium: Metallurgical and Materials Processing: Principles and Technologies; Materials Processing Fundamentals and New Technologies
Country/TerritoryUnited States
CitySan Diego, CA
Period2/03/036/03/03

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