High uptakes of CO2 and CH4 in mesoporous metal-organic frameworks MIL-100 and MIL-101

Philip L. Llewellyn; Sandrine Bourrelly; Christian Serre; Alexandre Vimont; Marco Daturi; Lomig Hamon; Guy De Weireld; Jong San Chang; Do Young Hong; Young Kyu Hwang; Sung Hwa Jhung; Gérard Férey

doi:10.1021/la800227x

High uptakes of CO₂ and CH₄ in mesoporous metal-organic frameworks MIL-100 and MIL-101

Philip L. Llewellyn
, Sandrine Bourrelly
, Christian Serre
, Alexandre Vimont
, Marco Daturi
, Lomig Hamon
, Guy De Weireld
, Jong San Chang
, Do Young Hong
, Young Kyu Hwang
, Sung Hwa Jhung
, Gérard Férey

Aix-Marseille Université
Institut Lavoisier de Versailles
UNICITE 14
Korea Research Institute of Chemical Technology
Universite de Mons

Research output: Contribution to journal › Article › peer-review

1137 Scopus citations

Abstract

Mesoporous MOFs MIL-100 and MIL-101 adsorb huge amounts of CO₂ and CH₄. Characterization was performed using both manometry and gravimetry in different laboratories for isotherms coupled with microcalorimetry and FTIR to specify the gas-solid interactions. In particular, the uptake of carbon dioxide in MIL-101 has been shown to occur with a record capacity of 40 mmol g^-1 or 390 cm³STp cm^-3 at 5 MPa and 303 K.

Original language	English
Pages (from-to)	7245-7250
Number of pages	6
Journal	Langmuir
Volume	24
Issue number	14
DOIs	https://doi.org/10.1021/la800227x
State	Published - 15 Jul 2008

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@article{8923ba36050f4f889578b3dffbec6b28,

title = "High uptakes of CO2 and CH4 in mesoporous metal-organic frameworks MIL-100 and MIL-101",

abstract = "Mesoporous MOFs MIL-100 and MIL-101 adsorb huge amounts of CO2 and CH4. Characterization was performed using both manometry and gravimetry in different laboratories for isotherms coupled with microcalorimetry and FTIR to specify the gas-solid interactions. In particular, the uptake of carbon dioxide in MIL-101 has been shown to occur with a record capacity of 40 mmol g-1 or 390 cm3STp cm-3 at 5 MPa and 303 K.",

author = "Llewellyn, \{Philip L.\} and Sandrine Bourrelly and Christian Serre and Alexandre Vimont and Marco Daturi and Lomig Hamon and \{De Weireld\}, Guy and Chang, \{Jong San\} and Hong, \{Do Young\} and Hwang, \{Young Kyu\} and Jhung, \{Sung Hwa\} and G{\'e}rard F{\'e}rey",

year = "2008",

month = jul,

day = "15",

doi = "10.1021/la800227x",

language = "English",

volume = "24",

pages = "7245--7250",

journal = "Langmuir",

issn = "0743-7463",

publisher = "American Chemical Society",

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TY - JOUR

T1 - High uptakes of CO2 and CH4 in mesoporous metal-organic frameworks MIL-100 and MIL-101

AU - Llewellyn, Philip L.

AU - Bourrelly, Sandrine

AU - Serre, Christian

AU - Vimont, Alexandre

AU - Daturi, Marco

AU - Hamon, Lomig

AU - De Weireld, Guy

AU - Chang, Jong San

AU - Hong, Do Young

AU - Hwang, Young Kyu

AU - Jhung, Sung Hwa

AU - Férey, Gérard

PY - 2008/7/15

Y1 - 2008/7/15

N2 - Mesoporous MOFs MIL-100 and MIL-101 adsorb huge amounts of CO2 and CH4. Characterization was performed using both manometry and gravimetry in different laboratories for isotherms coupled with microcalorimetry and FTIR to specify the gas-solid interactions. In particular, the uptake of carbon dioxide in MIL-101 has been shown to occur with a record capacity of 40 mmol g-1 or 390 cm3STp cm-3 at 5 MPa and 303 K.

AB - Mesoporous MOFs MIL-100 and MIL-101 adsorb huge amounts of CO2 and CH4. Characterization was performed using both manometry and gravimetry in different laboratories for isotherms coupled with microcalorimetry and FTIR to specify the gas-solid interactions. In particular, the uptake of carbon dioxide in MIL-101 has been shown to occur with a record capacity of 40 mmol g-1 or 390 cm3STp cm-3 at 5 MPa and 303 K.

UR - https://www.scopus.com/pages/publications/47949110984

U2 - 10.1021/la800227x

DO - 10.1021/la800227x

M3 - Article

AN - SCOPUS:47949110984

SN - 0743-7463

VL - 24

SP - 7245

EP - 7250

JO - Langmuir

JF - Langmuir

IS - 14

ER -

High uptakes of CO₂ and CH₄ in mesoporous metal-organic frameworks MIL-100 and MIL-101

Abstract

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