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Tunable kondo resonance at a pristine two-dimensional dirac semimetal on a kondo insulator

  • Jinwoong Hwang
  • , Seungseok Lee
  • , Ji Eun Lee
  • , Minhee Kang
  • , Hyejin Ryu
  • , Hyun Jeong Joo
  • , Jonathan Denlinger
  • , Jae Hoon Park
  • , Choongyu Hwang
  • Pusan National University
  • United States Department of Energy
  • Pohang University of Science and Technology
  • Korea Institute of Science and Technology

Research output: Contribution to journalArticlepeer-review

3 Scopus citations

Abstract

The proximity of two different materials leads to an intricate coupling of quasiparticles so that an unprecedented electronic state is often realized at the interface. Here, we demonstrate a resonance-type many-body ground state in graphene, a nonmagnetic two-dimensional Dirac semimetal, when grown on SmB6, a Kondo insulator, via thermal decomposition of fullerene molecules. This ground state is typically observed in three-dimensional magnetic materials with correlated electrons. Above the characteristic Kondo temperature of the substrate, the electron band structure of pristine graphene remains almost intact. As temperature decreases, however, the Dirac Fermions of graphene become hybridized with the Sm 4f states. Remarkable enhancement of the hybridization and Kondo resonance is observed with further cooling and increasing charge-carrier density of graphene, evidencing the Kondo screening of the Sm 4f local magnetic moment by the conduction electrons of graphene at the interface. These findings manifest the realization of the Kondo effect in graphene by the proximity of SmB6 that is tuned by the temperature and charge-carrier density of graphene.

Original languageEnglish
Pages (from-to)7973-7979
Number of pages7
JournalNano Letters
Volume20
Issue number11
DOIs
StatePublished - 11 Nov 2020

Keywords

  • ARPES
  • Graphene
  • Kondo effect
  • Proximity effect
  • SmB

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